Intuitive Model of Surface Modification Induced by Cluster Ion Beams

D Maciazek and M Kanski and Z Postawa, ANALYTICAL CHEMISTRY, 92, 7349-7353 (2020).

DOI: 10.1021/acs.analchem.0c01219

Topography development is one of the main factors limiting the quality of depth profiles during depth profiling experiments. One possible source of topography development is the formation of self-organized patterns due to cluster ion beam irradiation. In this work, we propose a simple model that can intuitively explain this phenomenon in terms of impact-induced mass transfer. By coupling our model with molecular dynamics simulations, we can predict the critical incidence angle, which separates the smoothening and roughening regimes. The results are in quantitative agreement with experiments. It is observed that the problems arising from topography development during depth profiling with cluster projectiles can be mitigated by reducing the beam incidence angle with respect to the surface normal or increasing its kinetic energy.

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