Relaxation Dynamics in the Energy Landscape of Glass-Forming Liquids

Y Nishikawa and M Ozawa and A Ikeda and P Chaudhuri and L Berthier, PHYSICAL REVIEW X, 12, 021001 (2022).

DOI: 10.1103/PhysRevX.12.021001

We numerically study the zero-temperature relaxation dynamics of several glass-forming models to their inherent structures, following quenches from equilibrium configurations sampled across a wide range of initial temperatures. In a mean-field Mari-Kurchan model, we find that relaxation changes from a power law to an exponential decay below a well-defined temperature, consistent with recent findings in mean-field p-spin models. By contrast, for finite-dimensional systems, the relaxation is always algebraic, with a nontrivial universal exponent at high temperatures crossing over to a harmonic value at low temperatures. We demonstrate that this apparent evolution is controlled by a temperature-dependent population of localized glassy excitations. Our work unifies several recent lines of studies aiming at a detailed characterization of the complex potential energy landscape of glass formers, and challenges both meanfield and real space descriptions of glasses.

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